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18B.12 Tarnishing of metal surfaces. In the oxidation of most metals (excluding the alkali andalkaline-earth metals) the volume of oxide produced is greater than that of the metal con-sumed. This oxide thus tends to form a compact film effectively insulating the oxygen andmetal from each other. For the derivations that follow it may be assumed that(a) For oxidation to proceed, oxygen must diffuse through the oxide film and that this diffusionfollows Fick's law.(b) The free surface of the oxide f
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